R movie > R the series: While I love a lot about R, the movie just feels so perfect and succinct and doesn't have some terrible plotlines like the breakup plot.
S the series >>>>>>>>>>>>> S movie: No offense, but the Princess Kaguya's Lover story is kinda meh in both the manga and the '90s anime.
SuperS Movie >>>>>>>>>>>>>>>>>>>>>>>>>> SuperS the series: This one is a no-brainer for me. Perle has more chemistry with Chibiusa in the 5 minutes they interacted than the entire 30 something episodes of Pegasus and Chibiusa (and he's not a horse!). The senshi seem way more competent in the movie and as much as people make a big deal about SuperS' animation, the movie completley blows it out of the water. The Outers appear. Chibi Moon has an actual attack. Did I mention no Horse x Little Girl romance?